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dc.contributor.authorFlorea, Larisaen
dc.contributor.authorDelaney, Colmen
dc.date.accessioned2020-04-17T13:17:15Z
dc.date.available2020-04-17T13:17:15Z
dc.date.issued2020en
dc.date.submitted2020en
dc.identifier.citationDanielle Bruen, Colm Delaney, Johnson Chung, Kalani Ruberu, Gordon G. Wallace, Dermot Diamond, Larisa Florea, 3D Printed Sugar-Sensing Hydrogels, Macromolecular Rapid Communications, 2020en
dc.identifier.otherYen
dc.identifier.urihttps://onlinelibrary.wiley.com/doi/abs/10.1002/marc.201900610
dc.identifier.urihttp://hdl.handle.net/2262/92311
dc.descriptionPUBLISHEDen
dc.description10.1002/marc.201900610en
dc.description.abstractThe ability of boronic acids to reversibly bind diols, such as sugars, has been widely studied in recent years. In solution, through the incorporation of additional fluorophores, this boronic acid-sugar interaction can be monitored by changes in fluorescence. Ultimately, a practical realization of this technology requires a transition from solution-based methodologies. Herein we present the first example of 3D printed sugar-sensing hydrogels, achieved through the incorporation of a boronic acid-fluorophore pair in a gelatin methacrylamide-based matrix. Through optimization of monomeric cocktails, it was possible to use extrusion printing to generate structured porous hydrogels which show a measurable and reproducible linear fluorescence response to glucose and fructose up to 100 mM.en
dc.language.isoenen
dc.relation.ispartofseriesMacromolecular Rapid Communicationsen
dc.rightsYen
dc.subjectHydrogelsen
dc.subjectBoronic aciden
dc.subject3D printingen
dc.subjectFluorescenceen
dc.title3D Printed Sugar-Sensing Hydrogelsen
dc.typeJournal Articleen
dc.contributor.sponsorScience Foundation Ireland (SFI)en
dc.contributor.sponsorAustralian Research Council (ARC)en
dc.contributor.sponsorEuropean Research Council (ERC)en
dc.contributor.sponsorScience Foundation Ireland (SFI)en
dc.contributor.sponsorScience Foundation Ireland (SFI)en
dc.type.supercollectionscholarly_publicationsen
dc.type.supercollectionrefereed_publicationsen
dc.identifier.peoplefinderurlhttp://people.tcd.ie/florealen
dc.identifier.peoplefinderurlhttp://people.tcd.ie/cdelane5en
dc.identifier.rssinternalid215751en
dc.identifier.doihttp://dx.doi.org/10.1002/marc.201900610en
dc.relation.ecprojectidinfo:eu-repo/grantAgreement/EC/FP7/802929
dc.rights.ecaccessrightsopenAccess
dc.contributor.sponsorGrantNumberSFI/12/RC/2289en
dc.contributor.sponsorGrantNumberCE 140100012en
dc.contributor.sponsorGrantNumber802929en
dc.contributor.sponsorGrantNumber16/TIDA/4183en
dc.contributor.sponsorGrantNumber12/RC/2278_2en
dc.subject.TCDThemeNanoscience & Materialsen
dc.subject.TCDThemeNext Generation Medical Devicesen
dc.subject.TCDTagBiopolymeric Materialsen
dc.subject.TCDTagHYDROGELen
dc.subject.TCDTagPHOTO-POLYMERISATIONen
dc.subject.TCDTagPOLYMERen
dc.subject.TCDTagPolymer Chemistryen
dc.subject.TCDTagSENSINGen
dc.subject.TCDTagsugar sensingen
dc.identifier.orcid_id0000-0002-4704-2393en
dc.status.accessibleNen


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